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            Free, publicly-accessible full text available June 1, 2026
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            Vera, Alexander; Zheng, Boyang; Yanez, Wilson; Yang, Kaijie; Kim, Seong Yeoul; Wang, Xinglu; Kotsakidis, Jimmy C; El-Sherif, Hesham; Krishnan, Gopi; Koch, Roland J; et al (, ACS Nano)A scalable platform to synthesize ultrathin heavy metals may enable high efficiency charge-to-spin conversion for next-generation spintronics. Here we report the synthesis of air-stable, epitaxially registered monolayer Pb underneath graphene on SiC (0001) by confinement heteroepitaxy (CHet). Diffraction, spectroscopy, and microscopy reveal CHet-based Pb intercalation predominantly exhibits a mottled hexagonal superstructure due to an ordered network of Frenkel-Kontorova-like domain walls. The system’s air stability enables ex-situ spin torque ferromagnetic resonance (ST-FMR) measurements that demonstrate charge-to-spin conversion in graphene/Pb/ferromagnet heterostructures with a 1.5× increase in the effective field ratio compared to control samples.more » « less
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            Wang, Qinqin; Xie, Ti; Blumenschein, Nicholas A.; Song, Zhihao; Kotsakidis, Jimmy C.; Hanbicki, Aubrey T.; Susner, Michael A.; Conner, Benjamin S.; Tan, Qishuo; Lee, Seng Huat; et al (, Matter)
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